<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys.net/inc/acp/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>8</volume_number>
		<issue_number>10</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/acp-8-2717-2008</doi>
	<article_url>http://www.atmos-chem-phys.net/8/2717/2008/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/8/2717/2008/acp-8-2717-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/8/2717/2008/acp-8-2717-2008.pdf</fulltext_pdf>
	<start_page>2717</start_page>
	<end_page>2728</end_page>
	<publication_date>2008-05-22</publication_date>
	<article_title content_type="html">Asian dust storm influence on North American ambient PM levels: observational evidence and controlling factors</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>T. L. Zhao</name>
		</author>
		<author numeration="2" affiliations="1,2">
			<name>S. L. Gong</name>
			<email>sunling.gong@ec.gc.ca</email>
		</author>
		<author numeration="3" affiliations="2">
			<name>X. Y. Zhang</name>
		</author>
		<author numeration="4" affiliations="3">
			<name>D. A. Jaffe</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Air Quality Research Division, Science and Technology Branch, Environment Canada, 4905 Dufferin Street, Toronto, Ontario, M3H 5T4, Canada</affiliation>
		<affiliation numeration="2" content_type="html">Centre for Atmosphere Watch and Services of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China</affiliation>
		<affiliation numeration="3" content_type="html">University of Washington-Bothell, 18115 Campus Way NE, Bothell, WA 98011-8246, USA</affiliation>
	</affiliations>
	<abstract content_type="html">New observational evidence of the trans-Pacific transport of Asian dust and
its contribution to the ambient particulate matter (PM) levels in North
America was revealed, based on the interannual variations between Asian dust
storms and the ambient PM levels in western North America from year 2000 to
2006. A high correlation was found between them with an &lt;I&gt;R&lt;/I&gt;&lt;sup&gt;2&lt;/sup&gt; value of
0.83. From analysis of the differences in the correlation between 2005 and
2006, three factors explain the variation of trans-Pacific transport and
influences of Asian dust storms on PM levels in western North America. These
were identified by modeling results and the re-analysis data. They were 1)
&lt;I&gt;Strength of frontal cyclones from Mongolia to north eastern
China&lt;/I&gt;: The frontal cyclones in East Asia not only bring strong cold air
outbreaks, generating dust storms in East Asia, but also lift Asian dust
into westerly winds of the free troposphere for trans-Pacific transport; 2)
&lt;I&gt;Pattern of transport pathway over the North Pacific&lt;/I&gt;: The
circulation patterns of westerlies over the North Pacific govern the
trans-Pacific transport pattern. Strong zonal airflow of the westerly jet in
the free troposphere over the North Pacific favor significant trans-Pacific
transport of Asian dust; 3) &lt;I&gt;Variation of precipitation in
the North Pacific&lt;/I&gt;: The scavenging of Asian dust particles by precipitation
is a major process of dust removal on the trans-Pacific transport pathway.
Therefore, variation of precipitation in the North Pacific could affect
trans-Pacific transport of Asian dust.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Arimoto, R., Kim, Y. J., Kim, Y. P., Quinn, P. K., Bates, T. S., Anderson, T. L., Gong, S., Uno, I., Chin, M., Huebert, B. J., Clarke, A. D., Shinozuka, Y., Weber, R. J., Anderson, J. R., Guazzotti, S. A., Sullivan, R. C., Sodeman, D. A., Prather, K. A., and Sokolik, I. N.: Characterization of Asian Dust during ACE-Asia, Global and Planet. Change, 52, 23&amp;ndash;56, doi:10.1016/j.gloplacha.2006.02.013, 2006. </reference>
		<reference numeration="2" content_type="text"> Bey, I., Jacob, D. J., Logan, J. A., and Yantosca, R. M.: Asian chemical outflow to the Pacific in spring: Origins, pathways, and budgets, J. Geophys. Res., 106, 23 097&amp;ndash;23 114, doi:10.1029/2001JD000806, 2001. </reference>
		<reference numeration="3" content_type="text"> Chun, Y., Boo, K.-O., Kim, J., Park, S.-U., and Lee, M.: Synopsis, transport and physical characteristics of Asian dust in Korea, J. Geophys. Res., 106, 18 461&amp;ndash;18 470, doi:10.1029/2001JD900184, 2001. </reference>
		<reference numeration="4" content_type="text"> Donnell, E. A., Fish, D. J., Dicks, E. M., and Thorpe, A. J.: Mechanisms for pollutant transport between the boundary layer and the free troposphere, J. Geophys. Res., 106, 7847&amp;ndash;7856, doi:10.1029/2000JD900730, 2001. </reference>
		<reference numeration="5" content_type="text"> Duce, R. A., Unni, C. K., Ray, B. J., Prospero, J. M., and Merrill, J. T.: Long-range atmospheric transport of soil dust from Asia to the tropical North Pacific: Temporal variability, Science, 209, 1,522&amp;ndash;1,524, 1980. </reference>
		<reference numeration="6" content_type="text"> Gong, S. L., Zhang, X. Y., Zhao, T. L., McKendry, I. G., Jaffe, D. A., and Lu, N. M.: Characterization Of Soil Dust Distributions In China And Its Transport During ACE-ASIA 2. Model Simulation and Validation, J. Geophys. Res., 108, 4262, doi:10.1029/2002JD002633, 2003. </reference>
		<reference numeration="7" content_type="text"> Gong, S. L., Zhang, X. Y., Zhao, T. L., Zhang, X. B., Barrie, L. A., McKendry, I. G., and Zhao, C. S.: A simulated climatology of Asian dust aerosol and its trans-Pacific transport. Part II: Interannual variability and climate connections, J. Climate, 19, 104&amp;ndash;122, 2006. </reference>
		<reference numeration="8" content_type="text"> Huebert, B. J., Bates, T., Russell, P. B., Shi, G., Kim, Y. J., Kawamura, K., Carmicheal, G. and Nakajima, T.: An overview of ACE-Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts, J. Geophys Res., 108, 8633, doi:10.1029/2003JD003550, 2003. </reference>
		<reference numeration="9" content_type="text"> Husar, R. B., Tratt, D. M., Schichtel, B. A., Falke, S. R., Li, F., Jaffe, D., Gassó, S., Gill, T., Laulainen, N. S., Lu, F., Reheis, M. C., Chun, Y., Westphal, D., Holben, B. N., Gueymard, C., McKendry, I., Kuring, N., Feldman, G. C., McClain, C., Frouin, R. J., Merrill, J., DuBois, D., Vignola, F., Murayama, T., Nickovic, S., Wilson, W. E., Sassen, K., Sugimoto, N., and Malm, W. C.: Asian dust evens of April 1998, J. Geophys. Res., 106, 18 317&amp;ndash;18 330, doi:10.1029/2000JD900788, 2001. </reference>
		<reference numeration="10" content_type="text"> Jaffe, D., McKendry, I., Anderson, T., and Price, H.: Six &quot;new&quot; episodes of trans-Pacific transport of air pollutants, Atmos. Environ., 37, 391&amp;ndash;404, 2003a. </reference>
		<reference numeration="11" content_type="text"> Jaffe, D. A., Anderson, T., Covert, D., Kotchenruther, R., Trost, B., Danielson, J., Simpson, W., Berntsen, T., Karlsdottir, S., Blake, D., Harris, J., Carmichael, G., and Uno, I.: Transport of Asian air pollution to North America, Geophys. Res. Lett., 26, 711&amp;ndash;714, doi:10.1029/1999GL900477, 1999. </reference>
		<reference numeration="12" content_type="text"> Jaffe, D. A., Snow, J., and Cooper, O.: The April 2001 Asian dust events: Transport and substantial impact on surface particulate matter concentrations across the United States, EOS Transactions, November 18, 2003b. </reference>
		<reference numeration="13" content_type="text"> Liang, Q., Jaeglé, L., Jaffe, D. A., Weiss-Penzias, P., Heckman, A., and Snow, J. A.: Long-range transport of Asian pollution to the northeast Pacific: Seasonal variations and transport pathways of carbon monoxide, J. Geophys. Res., 109, D23S07, doi:10.1029/2003JD004402, 2004. </reference>
		<reference numeration="14" content_type="text"> Liu, H., Jacob, D. J., Bey, R. M., Yantosca, R. M., Duncan, B. N., and Sachse, G. W.: Transport pathways for Asian pollution outflow over the Pacific: Interannual and seasonal variations, J. Geophys. Res., 108, 8786, doi:10.1029/2002JD003102, 2003. </reference>
		<reference numeration="15" content_type="text"> Mahowald, N., Luo, C., del Corral, J., and Zender, C. S.: Interannual variability in atmospheric mineral from a 22-year model simulation and observational data, J. Geophys. Res., 108, 4352, doi:10.1029/2002JD002821, 2003. </reference>
		<reference numeration="16" content_type="text"> Malm, W. C., Sisler, J. F., Huffman, D., Eldred, R. A., and Cahill, T. A.: Spatial and seasonal trends in particle concentration and optical extinction in the United States, J. Geophys. Res., 99, 1347&amp;ndash;1370, doi:10.1029/93JD02916, 1994. </reference>
		<reference numeration="17" content_type="text"> McKendry, I. G., Hacker, J. P., Stull, R., Sakiyama, S., Mignacca, D. and Reid, K.: Long-range transport of Asian dust to the Lower Fraser Valley, British Columbia, Canada, J. Geophys. Res., 106, 18 361&amp;ndash;18 370, doi:10.1029/2000JD900359, 2001. </reference>
		<reference numeration="18" content_type="text"> Merrill, J. T., Uematsu, M., and Bleck, R.: Meteorological analysis of long-range transport of mineral aerosols over the North Pacific, J. Geophys. Res., 94, 8584&amp;ndash;8598, 1989. </reference>
		<reference numeration="19" content_type="text"> Natsagdorj, L., Jugder, D., and Chung, Y. S.: Analysis of dust storms observed in Mongolia during 1937&amp;ndash;1999, Atmos. Environ., 37, 1401&amp;ndash;1411, 2003. </reference>
		<reference numeration="20" content_type="text"> Parrington, J. R., Zoller, W. H., and Aras, N. K.: Asian Dust: Seasonal Transport to the Hawaiian Islands, Science, 229, 195&amp;ndash;197, 1983. </reference>
		<reference numeration="21" content_type="text"> Prospero, J. M., Uematsu, M., and Savoie, D. L.: Mineral aerosol transport to the Pacific Ocean, in: Chemical Oceanography, edited by: Riley, J. P., Chester, R., and Duce, R. A., Academic, San Diego, CA, 188&amp;ndash;218, 1989. </reference>
		<reference numeration="22" content_type="text"> Qian, W., Quan, L., and Shi, S.: Variability of the dust storm in China and climatic control, J. Climate, 15, 1216&amp;ndash;1229, 2002. </reference>
		<reference numeration="23" content_type="text"> Seinfeld, J. H., Carmichael, G. R., Arimoto, R., Conant, W. C., Brechtel, F. J., Bates, T. S., Cahill, T. A., Clarke, A. D., Doherty, S. J., Flatau, P. J., Huebert, B. J., Kim, J., Markowicz, K. M., Quinn, P. K., Russell, L. M., Russell, P. B., Shimizu, A., Shinozuka, Y., Song, C. H., Tang, Y., Uno, I., Vogelmann, A. M., Weber, R. J., Woo, J. H., and Zhang, X. Y.: ACE-ASIA: Regional Climatic and Atmospheric Chemical Effects of Asian Dust and Pollution, B. Am. Meteorol. Soc., 85, 367&amp;ndash;380, 2004. </reference>
		<reference numeration="24" content_type="text"> Sun, J. M., Zhang, M. Y., and Liu, T. S.: Spatial and temporal characteristics of dust storms in China and its surrounding regions, 1960&amp;ndash;1999: Relations to source area and climate, J. Geophys. Res., 106, 10 325&amp;ndash;10 334, doi:10.1029/2000JD900665, 2001. </reference>
		<reference numeration="25" content_type="text"> Uematsu, M., Duce, R. A., Prospero, J. M., Chen, L., Merrill, J. T., and McDonald, R. L.: Transport of mineral aerosol from Asia over the North Pacific Ocean, J. Geophys. Res., 88, 5,343&amp;ndash;5,352, 1983. </reference>
		<reference numeration="26" content_type="text"> USEPA: Impact of April 2001 Asian dust event on particulate matter concentrations in the United States, National Air Quality and Emissions Trends Report, USEPA (US Environmental Protection Agency), Washington, D.C., 2003. </reference>
		<reference numeration="27" content_type="text"> VanCuren, R. A.: Asian aerosols in North America: Extracting the chemical composition and mass concentration of the Asian continental aerosol plume from long-term aerosol records in the western United States, J. Geophys. Res., 108, 4623, doi:10.1029/2003JD003459, 2003. </reference>
		<reference numeration="28" content_type="text"> VanCuren, R. A. and Cahill, T. A.: Asian aerosols in North America: Frequency and concentration of fine dust, J. Geophys. Res., 107, 4804, doi:10.1029/2002JD002204, 2002. </reference>
		<reference numeration="29" content_type="text"> VanCuren, R. A., Cliff, S. S., Perry, K. D., and Jimenez-Cruz, M.: Asian continental aerosol persistence above the marine boundary layer over the eastern North Pacific: Continuous aerosol measurements from Intercontinental Transport and Chemical Transformation 2002 (ITCT 2K2), J. Geophys. Res., 110, D09S90, doi:10.1029/2004JD004973, 2005. </reference>
		<reference numeration="30" content_type="text"> Wang, Y. Q., Zhang, X. Y., Gong, S. L., Zhou, C. H., Hu, X. Q., Liu, H. L., Niu, T., and Yang, Y. Q.: Surface observation of sand and dust storm in East Asia and its application in CUACE/Dust forecasting system, Atmos. Chem. Phys., 8, 545&amp;ndash;553, 2008. </reference>
		<reference numeration="31" content_type="text"> Wilkening, K. E., Barrie, L. A., and Engle, M.: Trans-Pacific air pollution, Science, 290, 65&amp;ndash;67, 2000. </reference>
		<reference numeration="32" content_type="text"> Xuan, J., Sokolikb, I. N., Hao, J., Guo, F., Mao, H., and G., Y.: Identification and characterization of sources of atmospheric mineral dust in East Asia, Atmos. Environ., 38, 6239&amp;ndash;6252, 2004. </reference>
		<reference numeration="33" content_type="text"> Yang, Y. Q., Hou, Q., Zhou, C. H., Liu, H. L., Wang, Y. Q., and Niu, T.: Sand/dust storm processes in Northeast Asia and associated large-scale circulations, Atmos. Chem. Phys., 8, 25&amp;ndash;33, 2008. </reference>
		<reference numeration="34" content_type="text"> Zhang, X. Y., An, Z. S., and Cao, J. J.: Dust emission from Chinese desert sources linked to variations in atmospheric circulation, J. Geophys. Res., 102, 28 041&amp;ndash;28 047, doi:10.1029/97JD02300, 1997. </reference>
		<reference numeration="35" content_type="text"> Zhang, X. Y., Arimoto, R., and An, Z. S.: Glacial and interglacial patterns for Asian dust transport, Quart. Sci. Rev., 18, 811&amp;ndash;819, 1999. </reference>
		<reference numeration="36" content_type="text"> Zhang, X. Y., Gong, S. L., Zhao, T. L., Arimoto, R., Wang, Y. Q., and Zhou, Z. J.: Sources of Asian dust and role of climate change versus desertification in Asian dust emission, Geophys. Res. Lett., 30, 2272, doi:10.1029/2003GL018206, 2003. </reference>
		<reference numeration="37" content_type="text"> Zhao, C., Dabu, X., and Li, Y.: Relationship between climatic factors and dust storm frequency in the Inner Mongolia of China, Geophys. Res. Lett., 31, L01103, doi:10.1029/2003GRL018206, 2004. </reference>
		<reference numeration="38" content_type="text"> Zhao, T. L., Gong, S. L., Zhang, X. Y., Blanchet, J. P., McKendry, I. G., and Zhou, Z. J.: A simulated climatology of Asian dust aerosol and its trans-Pacific transport. Part I: Mean climate and validation, J. Climate, 19, 88&amp;ndash;103, 2006. </reference>
		<reference numeration="39" content_type="text"> Zhao, T. L., Gong, S. L., Zhang, X. Y., and Mckendry, I. G.: Modeled size-segregated wet and dry deposition budgets of soil dust aerosol during ACE-Asia 2001: Implications for trans-Pacific transport, J. Geophys. Res., 108, 8665, doi:10.1029/2002JD003363, 2003. </reference>
		<reference numeration="40" content_type="text"> Zhou, C. H., Gong, S. L., Zhang, X. Y., Wang, Y. Q., Niu, T., Liu, H. L., Zhao, T. L., Yang, Y. Q., and Hou, Q.: Development and Evaluation of an Operational SDS Forecasting System for East Asia: CUACE/Dust, Atmos. Chem. Phys., 8, 787&amp;ndash;798, 2008. </reference>
		<reference numeration="41" content_type="text"> Zhou, Z. J.: Blowing-sand and sandstorm in China in recent 45 years, Quat. Sci., 21, 9&amp;ndash;17, 2001 (in Chinese). </reference>
	</references>
</article>

